Accessing Beyond-Light Line Dispersion and High-Q Resonances of Dense Plasmon Lattices by Bandfolding

Dense plasmon lattices are promising as experimentally accessible implementations of seminal tight-binding Hamiltonians, but the plasmonic dispersion of interest lies far beyond the light line and is thereby inaccessible in far-field optical experiments. In this work, we make the guided mode dispersion of dense hexagonal plasmon antenna lattices visible by bandfolding induced by perturbative scatterer size modulations that introduce supercell periodicity. We present fluorescence enhancement experiments and reciprocity-based T-matrix simulations for a systematic variation of perturbation strength. We evidence that folding the K-point into the light cone gives rise to a narrow plasmon mode, achieving among the highest reported quality factors for plasmon lattice resonances in the visible wavelength range despite a doubled areal density of plasmon antennas. We finally show K-point lasing and spontaneous symmetry breaking between the bandfolded K- and K′-modes, signifying that intrinsic symmetry properties of the dense plasmon lattice are maintained and can be observed upon band folding.