Active particle in a very thin interfacial droplet

A single light-driven Janus particle confined in a very thin oil droplet at an air-water interface displays intriguing dynamics. While laser activation induces rapid horizontal motion (1mm/s-1cm/s) by thermal Marangoni flow, the particle exhibits unexpected periodic circular motions or intermittent irregular motions. We show that the trajectories are the result of a coupling between the self-propulsion of the particle and the spatiotemporal droplet thickness changes. We propose a simple model where the properties of the active particle trajectories are governed by capillary forces and torques due to the confinement of the particle in the thin droplet.