Observation of Cooperative Purcell Enhancements in Antenna-Cavity Hybrids

Open Access
Authors
  • H.M. Doeleman
  • C.D. Dieleman
  • C. Mennes
  • B. Ehrler
Publication date 22-09-2020
Journal ACS Nano
Volume | Issue number 14 | 9
Pages (from-to) 12027-12036
Number of pages 10
Organisations
  • Faculty of Science (FNWI) - Institute of Physics (IoP) - Van der Waals-Zeeman Institute (WZI)
Abstract

Localizing light to nanoscale volumes through nanoscale resonators that are low loss and precisely tailored in spectrum to properties of matter is crucial for classical and quantum light sources, cavity QED, molecular spectroscopy, and many other applications. To date, two opposite strategies have been identified: to use either plasmonics with deep subwavelength confinement yet high loss and very poor spectral control or instead microcavities with exquisite quality factors yet poor confinement. In this work we realize hybrid plasmonic-photonic resonators that enhance the emission of single quantum dots, profiting from both plasmonic confinement and microcavity quality factors. Our experiments directly demonstrate how cavity and antenna jointly realize large cooperative Purcell enhancements through interferences. These can be controlled to engineer arbitrary Fano lineshapes in the local density of optical states.

Document type Article
Note With supplementary file
Language English
Published at https://doi.org/10.1021/acsnano.0c05233
Other links https://www.scopus.com/pages/publications/85091582177
Downloads
acsnano.0c05233 (Final published version)
Supplementary materials
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