Static and dynamical signatures of Dzyaloshinskii-Moriya interactions in the Heisenberg model on the kagome lattice

Open Access
Authors
  • D. Poilblanc
  • F. Becca
Publication date 06-2023
Journal SciPost Physics
Article number 139
Volume | Issue number 14 | 6
Number of pages 25
Organisations
  • Faculty of Science (FNWI) - Institute of Physics (IoP)
  • Faculty of Science (FNWI) - Institute of Physics (IoP) - Institute for Theoretical Physics Amsterdam (ITFA)
  • Faculty of Science (FNWI) - Institute of Physics (IoP) - Van der Waals-Zeeman Institute (WZI)
Abstract
Motivated by recent experiments on Cs2Cu3SnF12 and YCu3(OH)6Cl3, we consider the S = 1/2 Heisenberg model on the kagome lattice with nearest-neighbor superexchange J and (out-of-plane) Dzyaloshinskii-Moriya interaction JD, which favors (in-plane) Q = (0, 0) magnetic order. By using both variational Monte Carlo and tensor-network approaches, we show that the ground state develops a finite magnetization for J/ J ≳ 0.03−0.04; instead, for smaller values of the Dzyaloshinskii-Moriya interaction, the ground state has no magnetic order and, according to the fermionic wave function, develops a gap in the spinon spectrum, which vanishes for JD → 0. The small value of J/ J for the onset of magnetic order is particularly relevant for the interpretation of low-temperature behaviors of kagome antiferromagnets, including ZnCu3(OH)6Cl2. For this reason, we assess the spin dynamical structure factor and the corresponding low-energy spectrum, by using the variational Monte Carlo technique. The existence of a continuum of excitations above the magnon modes is observed within the magnetically ordered phase, with a broad peak above the lowest-energy magnons, similarly to what has been detected by inelastic neutron scattering on Cs2Cu3SnF12.
Document type Article
Language English
Published at https://doi.org/10.21468/SciPostPhys.14.6.139
Other links https://www.scopus.com/pages/publications/85163381233
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SciPostPhys_14_6_139 (Final published version)
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