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Zoekopdracht: journal id: "physicalxreviewxletters"

AuteursM. Sovago, R.K. Campen, G.W.H. Wurpel, M. Müller, H.J. Bakker, M. Bonn
TitelVibrational response of hydrogen-bonded interfacial water is dominated by intramolecular coupling
TijdschriftPhysical Review Letters
Jaargang100
Jaar2008
Nummer17
Pagina's173901-
ISSN00319007
FaculteitFaculteit der Natuurwetenschappen, Wiskunde en Informatica
Instituut/afd.FNWI: Van 't Hoff Institute for Molecular Sciences (HIMS)
FNWI: Swammerdam Institute for Life Sciences (SILS)
SamenvattingUsing the surface-specific vibrational technique of vibrational sum-frequency generation, we reveal that the double-peaked structure in the vibrational spectrum of hydrogen-bonded interfacial water molecules originates from vibrational coupling between the stretch and bending overtone, rather than from structural effects. This is demonstrated by isotopic dilution experiments, which reveal a smooth transition from two peaks to one peak, as D2O is converted into HDO. Our results show that the water interface is structurally more homogeneous than previously thought.
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