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Query: faculty: "FNWI" and publication year: "2009"

AuthorsP.A.R. Breuil, F.W. Patureau, J.N.H. Reek
TitleSingly hydrogen bonded supramolecular ligands for highly selective rhodium-catalyzed hydrogenation reactions
JournalAngewandte Chemie, International Edition
Volume48
Year2009
Issue12
Pages2162-2165
ISSN14337851
FacultyFaculty of Science
Institute/dept.FNWI: Van 't Hoff Institute for Molecular Sciences (HIMS)
AbstractH bonds make the catalysts! A single hydrogen bond between ligands coordinated to a rhodium center is critical for the formation of pure supramolecular catalysts for asymmetric hydrogenation reactions. The ester group of the amidite ligand (see scheme) also forms a hydrogen bond with the coordinated substrate. Use of the heterocomplex afforded the highest enantioselectivity reported to date for the hydrogenation of several ester substrates.
Document typeArticle
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