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Zoekopdracht: faculteit: "FNWI" en publicatiejaar: "1997"

AuteursJ.B. Milan, W.J. Buma, C.A. de Lange, K. Wang, V. McKoy
TitelRotationally resolved multiphoton ionization photoelectron spectroscopy of the [a 1D]3dp 2F and [a 1D]5pp 2F Rydberg states of the SH radical
TijdschriftThe Journal of Chemical Physics
FaculteitFaculteit der Natuurwetenschappen, Wiskunde en Informatica
Instituut/afd.FNWI: Van 't Hoff Institute for Molecular Sciences (HIMS)
TrefwoordenRydberg states; mercapto radical; ab initio calculations; REMPI-PES
Basisclassificatie33.33 ; 35.11 ; 35.25
SamenvattingExperimental and theoretical results on the rotationally resolved photoelectron spectra of the [a 1]3d 2(v = 0) and the [a 1]5p 2(v = 0) Rydberg states of the SH radical are presented. In particular, for the former state, ionization via a large number of members of different rotational branches is considered. The interplay between experiment and ab initio calculations, including alignment, allows for a detailed interpretation of the results. Asymmetries apparent in the rotational ionic distributions and the observed suppression of transitions involving a large change in angular momentum can be explained on the basis of the theory. ©1997 American Institute of Physics.
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